Recent Advances of Transition Metal Chalcogenides as Cathode Materials for Aqueous Zinc-Ion Batteries.

In recent years, advances in lithium-ion batteries (LIBs) have pushed the research of other metal-ion batteries to the forefront. Aqueous zinc ion batteries (AZIBs) have attracted much attention owing to their low cost, high capacity and non-toxic characteristics. Among various cathodes, transition metal chalcogenides (TMCs) with a layered structure are considered as suitable electrode materials. The large layer spacing facilitates the intercalation/de-intercalation of Zn 2+ between the layers. In this mini-review, we summarize a variety of design strategies for the modification of TMCs. Then, we specifically emphasize the zinc storage capacity of the optimized electrodes. Finally, we propose the challenges and future prospects of cathode materials for high-energy AZIBs.