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Large anomalous Nernst effect and nodal plane in an iron-based kagome ferromagnet.

Taishi ChenSusumu MinamiAkito SakaiYangming WangZili FengTakuya NomotoMotoaki HirayamaRieko IshiiTakashi KoretsuneRyotaro AritaSatoru Nakatsuji
Published in: Science advances (2022)
Anomalous Nernst effect (ANE), converting a heat flow to transverse electric voltage, originates from the Berry phase of electronic wave function near the Fermi energy E F . Thus, the ANE provides a sensitive probe to detect a topological state that produces large Berry curvature. In addition, a magnet that exhibits a large ANE using low-cost and safe elements will be useful to develop a novel energy harvesting technology. Here, we report our observation of a high ANE exceeding 3 microvolts per kelvin above room temperature in the kagome ferromagnet Fe 3 Sn with the Curie temperature of 760 kelvin. Our theoretical analysis clarifies that a “nodal plane” produces a flat hexagonal frame with strongly enhanced Berry curvature, resulting in the large ANE. Our discovery of the large ANE in Fe 3 Sn opens the path for the previously unexplored functionality of flat degenerate electronic states and for developing flexible film thermopile and heat current sensors.
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