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Single-shot ultrafast terahertz photography.

Junliang DongPei YouAlessandro TomasinoAycan YurtseverRoberto Morandotti
Published in: Nature communications (2023)
Multidimensional imaging of transient events has proven pivotal in unveiling many fundamental mechanisms in physics, chemistry, and biology. In particular, real-time imaging modalities with ultrahigh temporal resolutions are required for capturing ultrashort events on picosecond timescales. Despite recent approaches witnessing a dramatic boost in high-speed photography, current single-shot ultrafast imaging schemes operate only at conventional optical wavelengths, being suitable solely within an optically-transparent framework. Here, leveraging on the unique penetration capability of terahertz radiation, we demonstrate a single-shot ultrafast terahertz photography system that can capture multiple frames of a complex ultrafast scene in non-transparent media with sub-picosecond temporal resolution. By multiplexing an optical probe beam in both the time and spatial-frequency domains, we encode the terahertz-captured three-dimensional dynamics into distinct spatial-frequency regions of a superimposed optical image, which is then computationally decoded and reconstructed. Our approach opens up the investigation of non-repeatable or destructive events that occur in optically-opaque scenarios.
Keyphrases
  • high speed
  • high resolution
  • atomic force microscopy
  • energy transfer
  • climate change
  • mass spectrometry
  • radiation therapy
  • quantum dots
  • electron transfer
  • living cells
  • psychometric properties
  • fluorescent probe