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Sources of black carbon to the Himalayan-Tibetan Plateau glaciers.

Chaoliu LiCarme BoschShichang KangAugust AnderssonPengfei ChenQianggong ZhangZhiyuan CongBing ChenDahe QinÖrjan Gustafsson
Published in: Nature communications (2016)
Combustion-derived black carbon (BC) aerosols accelerate glacier melting in the Himalayas and in Tibet (the Third Pole (TP)), thereby limiting the sustainable freshwater supplies for billions of people. However, the sources of BC reaching the TP remain uncertain, hindering both process understanding and efficient mitigation. Here we present the source-diagnostic Δ(14)C/δ(13)C compositions of BC isolated from aerosol and snowpit samples in the TP. For the Himalayas, we found equal contributions from fossil fuel (46±11%) and biomass (54±11%) combustion, consistent with BC source fingerprints from the Indo-Gangetic Plain, whereas BC in the remote northern TP predominantly derives from fossil fuel combustion (66±16%), consistent with Chinese sources. The fossil fuel contributions to BC in the snowpits of the inner TP are lower (30±10%), implying contributions from internal Tibetan sources (for example, yak dung combustion). Constraints on BC sources facilitate improved modelling of climatic patterns, hydrological effects and provide guidance for effective mitigation actions.
Keyphrases
  • mass spectrometry
  • high resolution
  • drinking water
  • particulate matter
  • sewage sludge
  • municipal solid waste
  • wastewater treatment
  • african american