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A metal-catalyzed thermal polymerization strategy toward atomically dispersed catalysts.

Lin-Wei ChenZhen-Yu WuHang NanLei WangSheng-Qi ChuHai-Wei Liang
Published in: Chemical communications (Cambridge, England) (2019)
We report a general metal-catalyzed thermal polymerization strategy for the preparation of atomically dispersed catalysts that consist of isolated metal atoms (Fe, Co and Ni) hosted by a polymer-like carrier containing phenanthroline substructure. The prepared atomically dispersed cobalt catalysts exhibit high selectivity, activity, and reusability in catalyzing aromatic alkane oxidation.
Keyphrases
  • metal organic framework
  • highly efficient
  • transition metal
  • room temperature
  • high resolution
  • nitric oxide
  • molecularly imprinted