A Ternary Pt/Au/TiO2 -Decorated Plasmonic Wood Carbon for High-Efficiency Interfacial Solar Steam Generation and Photodegradation of Tetracycline.
Minmin WangPing WangJie ZhangChuanping LiYongdong JinPublished in: ChemSusChem (2019)
A ternary Pt/Au/TiO2 nanoparticle (NP) decorated plasmonic wood carbon has been successfully fabricated by a simple two-step calcination method. The as-prepared Pt/Au/TiO2 NP-decorated wood carbon showed an interfacial solar steam generation efficiency up to 90.4 %. Furthermore, the floating system exhibits an excellent photodegradation of tetracycline (TC; 40 mg L-1 ). Up to 94 % degradation was achieved after 80 min of continuous light irradiation (λ>420 nm) with the assistance of solar steam process. The photocatalysis is promoted by the introduction of Pt/Au nanocomponents, which suppress the recombination of electron-hole pairs generated on TiO2 and facilitate electron transfer. High-performance liquid chromatography mass spectrometry was employed to identify the reaction products of the photocatalytic system and a mechanistic insight was also provided. The as-prepared three-dimensional plasmonic wood carbon has a high photocatalytic performance. Such wood carbon-based system is recyclable and scalable for practical and versatile solar-driven clean water generation.
Keyphrases
- visible light
- electron transfer
- high performance liquid chromatography
- mass spectrometry
- high efficiency
- reduced graphene oxide
- ionic liquid
- high resolution
- dna damage
- solid phase extraction
- photodynamic therapy
- quantum dots
- sensitive detection
- gold nanoparticles
- radiation therapy
- single molecule
- oxidative stress
- gas chromatography