Reflective dielectric cavity enhanced emission from hexagonal boron nitride spin defect arrays.
Xiao-Dong ZengYuan-Ze YangNai-Jie GuoZhi-Peng LiZhao-An WangLin-Ke XieShang YuYu MengQiang LiJin-Shi XuWei LiuYi-Tao WangJian-Shun TangChuan-Feng LiGuang-Can GuoPublished in: Nanoscale (2023)
Among the various kinds of spin defects in hexagonal boron nitride (hBN), the negatively charged boron vacancy (V B - ) spin defect that can be site-specifically generated is undoubtedly a potential candidate for quantum sensing, but its low quantum efficiency restricts its practical applications. Here, we demonstrate a robust enhancement structure called reflective dielectric cavity (RDC) with advantages including easy on-chip integration, convenient processing, low cost and suitable broad-spectrum enhancement for V B - defects. In the experiment, we used a metal reflective layer under the hBN flakes, filled with a transition dielectric layer in the middle, and adjusted the thickness of the dielectric layer to achieve the best coupling between RDC and spin defects in hBN. A remarkable 11-fold enhancement in the fluorescence intensity of V B - spin defects in hBN flakes can be achieved. By designing the metal layer into a waveguide structure, high-contrast optically detected magnetic resonance (ODMR) signal (∼21%) can be obtained. The oxide layer of the RDC can be used as the integrated material to implement secondary processing of micro-nano photonic devices, which means that it can be combined with other enhancement structures to achieve stronger enhancement. This work has guiding significance for realizing the on-chip integration of spin defects in two-dimensional materials.