Measuring Spin⋅⋅⋅Spin Interactions between Heterospins in a Hybrid [2]Rotaxane.

Marie-Emmanuelle BoulonAntonio FernandezEufemio Moreno Pineda Nicholas F ChiltonGrigore TimcoAlistair J Fielding Richard E P Winpenny

Published in: Angewandte Chemie (International ed. in English) (2017)

Use of molecular electron spins as qubits for quantum computing will depend on the ability to produce molecules with weak but measurable interactions between the qubits. Here we demonstrate use of pulsed EPR spectroscopy to measure the interaction between two inequivalent spins in a hybrid rotaxane molecule.

Keyphrases

single molecule
room temperature
density functional theory
molecular dynamics
high resolution
transition metal
energy transfer
solid state
solar cells
monte carlo