Field-free switching of perpendicular magnetization by two-dimensional PtTe 2 /WTe 2 van der Waals heterostructures with high spin Hall conductivity.

The key challenge of spin-orbit torque applications lies in exploring an excellent spin source capable of generating out-of-plane spins while exhibiting high spin Hall conductivity. Here we combine PtTe 2 for high spin conductivity and WTe 2 for low crystal symmetry to satisfy the above requirements. The PtTe 2 /WTe 2 bilayers exhibit a high in-plane spin Hall conductivity σ s,y  ≈ 2.32 × 10 5  × ħ/2e Ω -1  m -1 and out-of-plane spin Hall conductivity σ s,z  ≈ 0.25 × 10 5  × ħ/2e Ω -1  m -1 , where ħ is the reduced Planck's constant and e is the value of the elementary charge. The out-of-plane spins in PtTe 2 /WTe 2 bilayers enable the deterministic switching of perpendicular magnetization at room temperature without magnetic fields, and the power consumption is 67 times smaller than that of the Pt control case. The high out-of-plane spin Hall conductivity is attributed to the conversion from in-plane spin to out-of-plane spin, induced by the crystal asymmetry of WTe 2 . Our work establishes a low-power perpendicular magnetization manipulation based on wafer-scale two-dimensional van der Waals heterostructures.