Rational Drug Design of Topically Administered Caspase 1 Inhibitors for the Treatment of Inflammatory Acne.
Jean-François FournierLaurence ClarySandrine ChambonLaurence DumaisCraig Steven HarrisCorinne MilloisRomain PierreSandrine TalanoÉtienne ThoreauJérome AubertMichèle AurellyClaire Bouix-PeterAnne BrethonLaurent ChantalatOlivier ChristinCatherine CominoGhizlane El-BazbouzAnne-Laurence GhiliniTatiana IsabetClaude LardyAnne-Pascale LuzyCéline MathieuKenny MebroukDanielle OrfilaJonathan PascauKevin ReverseDidier RocheVincent RodeschiniLaurent François HennequinPublished in: Journal of medicinal chemistry (2018)
The use of an interleukin β antibody is currently being investigated in the clinic for the treatment of acne, a dermatological disorder affecting 650M persons globally. Inhibiting the protease responsible for the cleavage of inactive pro-IL1β into active IL-1β, caspase-1, could be an alternative small molecule approach. This report describes the discovery of uracil 20, a potent (38 nM in THP1 cells assay) caspase-1 inhibitor for the topical treatment of inflammatory acne. The uracil series was designed according to a published caspase-1 pharmacophore model involving a reactive warhead in P1 for covalent reversible inhibition and an aryl moiety in P4 for selectivity against the apoptotic caspases. Reversibility was assessed in an enzymatic dilution assay or by using different substrate concentrations. In addition to classical structure-activity-relationship exploration, topical administration challenges such as phototoxicity, organic and aqueous solubility, chemical stability in solution, and skin metabolic stability are discussed and successfully resolved.
Keyphrases
- cell death
- induced apoptosis
- small molecule
- high throughput
- oxidative stress
- primary care
- signaling pathway
- combination therapy
- emergency department
- anti inflammatory
- systematic review
- cell cycle arrest
- endoplasmic reticulum stress
- hidradenitis suppurativa
- wound healing
- liquid chromatography tandem mass spectrometry
- molecular dynamics
- high resolution
- replacement therapy
- amino acid