Efficient generation of entangled multiphoton graph states from a single atom.

The central technological appeal of quantum science resides in exploiting quantum effects, such as entanglement, for a variety of applications, including computing, communication and sensing 1 . The overarching challenge in these fields is to address, control and protect systems of many qubits against decoherence 2 . Against this backdrop, optical photons, naturally robust and easy to manipulate, represent ideal qubit carriers. However, the most successful technique so far for creating photonic entanglement 3 is inherently probabilistic and, therefore, subject to severe scalability limitations. Here we report the implementation of a deterministic protocol 4-6 for the creation of photonic entanglement with a single memory atom in a cavity 7 . We interleave controlled single-photon emissions with tailored atomic qubit rotations to efficiently grow Greenberger-Horne-Zeilinger (GHZ) states 8 of up to 14 photons and linear cluster states 9 of up to 12 photons with a fidelity lower bounded by 76(6)% and 56(4)%, respectively. Thanks to a source-to-detection efficiency of 43.18(7)% per photon, we measure these large states about once every minute, which is orders of magnitude faster than in any previous experiment 3,10-13 . In the future, this rate could be increased even further, the scheme could be extended to two atoms in a cavity 14,15 or several sources could be quantum mechanically coupled 16 , to generate higher-dimensional cluster states 17 . Overcoming the limitations encountered by probabilistic schemes for photonic entanglement generation, our results may offer a way towards scalable measurement-based quantum computation 18,19 and communication 20,21 .