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Genome Mining of Streptomyces mobaraensis DSM40847 as a Bleomycin Producer Providing a Biotechnology Platform To Engineer Designer Bleomycin Analogues.

null HindraDong YangQihui TengLiao-Bin DongIvana CrnovčićTingting HuangHuiming GeBen Shen
Published in: Organic letters (2017)
Streptomyces mobaraensis DSM40847 has been identified by genome mining and confirmed to be a new bleomycin (BLM) producer. Manipulation of BLM biosynthesis in S. mobaraensis has been demonstrated, as exemplified by the engineered production of 6'-deoxy-BLM A2, providing a biotechnology platform for BLM biosynthesis and engineering. Comparison of DNA cleavage efficiency and kinetics among 6'-deoxy-BLM A2 and selected analogues supports the wisdom of altering the disaccharide moiety to fine-tune BLM activity.
Keyphrases
  • pulmonary fibrosis
  • high throughput
  • molecular docking
  • single molecule
  • cell wall
  • structure activity relationship