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Ruthenium-Catalyzed Pyridine-Directed Aryl C-H Glycosylation with Glycosyl Chlorides.

Shaokun CaiQikai SunQuanquan WangGang HeGong Chen
Published in: The Journal of organic chemistry (2022)
Metal-catalyzed C - H glycosylation reactions with glycosyl chloride donors have emerged as a useful strategy for the synthesis of C -glycosides. Previously, palladium and nickel complexes were reported to catalyze C - H glycosylation reactions using amide-linked bidentate auxiliaries. Herein, a ruthenium-catalyzed ortho C - H glycosylation reaction of arenes with various glycosyl chloride donors using a monodentate pyridine directing group is developed. Preliminary mechanistic studies indicated that two-electron oxidative addition and reductive elimination of ruthenocycle intermediate led to the glycosylation products.
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