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Stereoselective Synthesis of Maresin-like Lipid Mediators.

Song HongYan LuMasao MoritaShun SaitoYuichi KobayashiBokkyoo JunNicolas G BazanXiaoming XuYapin Wang
Published in: Synlett : accounts and rapid communications in synthetic organic chemistry (2019)
Maresin-L1 (14S,22-dihydroxy-docosa-4Z,7Z,10Z,12E,16Z,19Z-hexaenoic acid) and maresin-L2 (14R,22-dihydroxy-docosa-4Z,7Z,10Z,12E,16Z,19Z-hexaenoic acid) were chemically synthesized. They were identical to activated macrophage produced counterparts and their total synthesis was highly Stereoselective, as revealed by chiral LC-UV-MS/MS analysis. The synthesis involved the following steps: (1) kinetic resolution of a racemic allylic alcohol by the asymmetric epoxidation; (2) transformation of the epoxy alcohol to γ-hydroxyenal derivative; and (3) the Wittig reaction to furnish the Z-olefin.
Keyphrases
  • ms ms
  • mass spectrometry
  • ionic liquid
  • fatty acid
  • liquid chromatography tandem mass spectrometry
  • electron transfer
  • aqueous solution